A few different things can cause spasms. The one you already mentioned is calcium deficiency. Spasms can also occur from liver and kidney failure. The fact that the spasms occur rapidly in succession does not bode well. Possibly problems include:
Metabolic Bone Disease/Calcium deficiency: get him eating leafy greens that are high in calcium such as mustard greens, collard greens, turnip greens and endive. If you have it, dust his greens with calcium CITRATE as it is more readily assimilated in herbiverous lizards. (Carbonate is assimilated well only if taken with protein such as crickets). If he is not completely stressed by the move: ie eating, try and give him some natural sunlight. Make sure you have an excellent UVB source such as a mercury vapor bulb.
Kidney Failure: Were his previous owners feeding him crickets? Kidney failure is common in herbivorous lizards that are fed animal protein. Stay away from crickets, mealworms or any other source of animal protein. Also, he may be dehydrated which causes more stress on the kidneys. Drip some water on his snout and see if he drinks and/or give him a 15 minute soak.
Liver Failure: Liver failure is usually a side effect of kidney failure as the kidneys transfer unprocessed toxins to the liver. Is this Mali a fresh import? Oftentimes distributors that sell imported animals will administer deworming medication themselves without consulting a vet. An overdose of medication can cause liver failure.
And remember, if it gets worse take him to see a vet as soon as possible. Hope he gets better,
Peter